Application of the pitzer method for modeling densities of actinide solutions in the scale code system

Charles F. Weber; Calvin M. Hopper

doi:10.13182/NT06-A3684

Application of the pitzer method for modeling densities of actinide solutions in the scale code system

Charles F. Weber
, Calvin M. Hopper

Collection Science and Engineering

Research output: Contribution to journal › Article › peer-review

8 Scopus citations

Abstract

A new approach to modeling fissile solution densities is developed and applied to arbitrary solutions of UO₂²⁺, Th⁴⁺, Pu⁴⁺, H⁺, and NO₃ ^- in water. The model is based on the semiempirical method of Pitzer for describing electrolyte solution thermodynamics. This new density model has been included in the recent release of the SCALE 5 code system as the default for criticality calculations of fissile solutions.

Original language	English
Pages (from-to)	1-8
Number of pages	8
Journal	Nuclear Technology
Volume	153
Issue number	1
DOIs	https://doi.org/10.13182/NT06-A3684
State	Published - Jan 2006

Keywords

Partial molar volume
Thorium nitrate
Uranyl nitrate

Access to Document

10.13182/NT06-A3684

Cite this

@article{edc144ffe8e549e8b47fb3ab8b3d25fa,

title = "Application of the pitzer method for modeling densities of actinide solutions in the scale code system",

abstract = "A new approach to modeling fissile solution densities is developed and applied to arbitrary solutions of UO22+, Th4+, Pu4+, H+, and NO3 - in water. The model is based on the semiempirical method of Pitzer for describing electrolyte solution thermodynamics. This new density model has been included in the recent release of the SCALE 5 code system as the default for criticality calculations of fissile solutions.",

keywords = "Partial molar volume, Thorium nitrate, Uranyl nitrate",

author = "Weber, \{Charles F.\} and Hopper, \{Calvin M.\}",

year = "2006",

month = jan,

doi = "10.13182/NT06-A3684",

language = "English",

volume = "153",

pages = "1--8",

journal = "Nuclear Technology",

issn = "0029-5450",

publisher = "Taylor and Francis Group",

number = "1",

}

TY - JOUR

T1 - Application of the pitzer method for modeling densities of actinide solutions in the scale code system

AU - Weber, Charles F.

AU - Hopper, Calvin M.

PY - 2006/1

Y1 - 2006/1

N2 - A new approach to modeling fissile solution densities is developed and applied to arbitrary solutions of UO22+, Th4+, Pu4+, H+, and NO3 - in water. The model is based on the semiempirical method of Pitzer for describing electrolyte solution thermodynamics. This new density model has been included in the recent release of the SCALE 5 code system as the default for criticality calculations of fissile solutions.

AB - A new approach to modeling fissile solution densities is developed and applied to arbitrary solutions of UO22+, Th4+, Pu4+, H+, and NO3 - in water. The model is based on the semiempirical method of Pitzer for describing electrolyte solution thermodynamics. This new density model has been included in the recent release of the SCALE 5 code system as the default for criticality calculations of fissile solutions.

KW - Partial molar volume

KW - Thorium nitrate

KW - Uranyl nitrate

UR - https://www.scopus.com/pages/publications/30844435009

U2 - 10.13182/NT06-A3684

DO - 10.13182/NT06-A3684

M3 - Article

AN - SCOPUS:30844435009

SN - 0029-5450

VL - 153

SP - 1

EP - 8

JO - Nuclear Technology

JF - Nuclear Technology

IS - 1

ER -

Application of the pitzer method for modeling densities of actinide solutions in the scale code system

Abstract

Keywords

Access to Document

Other files and links

Fingerprint

Cite this