An innovative carbonated cementitious material and its printability and carbon mineralization capacity

Paula Bran Anleu; Yann Le Pape; Qiyi Chen; Rigoberto Advincula; Xiao Guang Sun; Justin B. Felder; Harry M. Meyer; Brian K. Post; Michael J. Lance; M. Parans Paranthaman

doi:10.1007/s40964-023-00463-2

An innovative carbonated cementitious material and its printability and carbon mineralization capacity

Paula Bran Anleu, Yann Le Pape, Qiyi Chen, Rigoberto Advincula, Xiao Guang Sun, Justin B. Felder, Harry M. Meyer, Brian K. Post, Michael J. Lance, M. Parans Paranthaman

Research output: Contribution to journal › Article › peer-review

3 Scopus citations

Abstract

The main goal of this research is to develop a carbonated cementitious material (CCMs) mix design and demonstrate its rapid stiffening for manufacturing 3D printed or precast elements for building construction (i.e., concrete with enhanced durability and CO₂ capture efficiency). The material development employs hydrated Ca(OH)₂, and its distinct reaction with CO₂ to form CaCO₃. Different formulations and additives including polymer materials enable the thermomechanical properties that give these CCMs 3D printability comparable with cement materials used for similar applications. Printable and castable CCM formulations were successfully developed and demonstrated to mineralize CO₂ to form up to 57% CaCO₃.

Original language	English
Pages (from-to)	435-444
Number of pages	10
Journal	Progress in Additive Manufacturing
Volume	9
Issue number	2
DOIs	https://doi.org/10.1007/s40964-023-00463-2
State	Published - Apr 2024

Funding

This research was supported by the Laboratory Directed Research & Development Seed Money Fund at the Oak Ridge National Laboratory. A portion of this research was carried out at the Center for Nanophase Materials Sciences, which is a US Department of Energy Office of Science User Facility. Access to the Raman spectrometer was provided by the Nuclear Nonproliferation Division, Oak Ridge National Laboratory. This manuscript has been authored by UT-Battelle LLC, under contract DE-AC05-00OR22725 with the US Department of Energy (DOE). The US government retains and the publisher, by accepting the article for publication, acknowledges that the US government retains a nonexclusive, paid-up, irrevocable, worldwide license to publish or reproduce the published form of this manuscript, or allow others to do so, for US government purposes. DOE will provide public access to these results of federally sponsored research in accordance with the DOE Public Access Plan ( http://energy.gov/downloads/doe-public-access-plan ).

Funders	Funder number
U.S. Department of Energy
Oak Ridge National Laboratory
Laboratory Directed Research and Development
UT-Battelle	DE-AC05-00OR22725

Keywords

3D printing
Calcium carbonate
Carbonation

UN SDGs

This output contributes to the following UN Sustainable Development Goals (SDGs)

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10.1007/s40964-023-00463-2

Cite this

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abstract = "The main goal of this research is to develop a carbonated cementitious material (CCMs) mix design and demonstrate its rapid stiffening for manufacturing 3D printed or precast elements for building construction (i.e., concrete with enhanced durability and CO2 capture efficiency). The material development employs hydrated Ca(OH)2, and its distinct reaction with CO2 to form CaCO3. Different formulations and additives including polymer materials enable the thermomechanical properties that give these CCMs 3D printability comparable with cement materials used for similar applications. Printable and castable CCM formulations were successfully developed and demonstrated to mineralize CO2 to form up to 57% CaCO3.",

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AU - Advincula, Rigoberto

AU - Sun, Xiao Guang

AU - Felder, Justin B.

AU - Meyer, Harry M.

AU - Post, Brian K.

AU - Lance, Michael J.

AU - Paranthaman, M. Parans

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AB - The main goal of this research is to develop a carbonated cementitious material (CCMs) mix design and demonstrate its rapid stiffening for manufacturing 3D printed or precast elements for building construction (i.e., concrete with enhanced durability and CO2 capture efficiency). The material development employs hydrated Ca(OH)2, and its distinct reaction with CO2 to form CaCO3. Different formulations and additives including polymer materials enable the thermomechanical properties that give these CCMs 3D printability comparable with cement materials used for similar applications. Printable and castable CCM formulations were successfully developed and demonstrated to mineralize CO2 to form up to 57% CaCO3.

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An innovative carbonated cementitious material and its printability and carbon mineralization capacity

Abstract

Funding

Keywords

UN SDGs

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