Age-dating methodology for 137Cs ceramic sources

Jennifer L. Steeb; Donald G. Graczyk; Yifen Tsai; Carol J. Mertz; Ashleigh Kimberlin; David B. Chamberlain

doi:10.1007/s10967-016-4712-x

Age-dating methodology for ¹³⁷Cs ceramic sources

Jennifer L. Steeb
, Donald G. Graczyk
, Yifen Tsai
, Carol J. Mertz
, Ashleigh Kimberlin
, David B. Chamberlain

Research output: Contribution to journal › Article › peer-review

8 Scopus citations

Abstract

Age-dating of ¹³⁷Cs ceramic sources is shown to be a viable technology for nuclear forensics investigations. The ¹³⁷Cs age-dating method in general, however, could be substantially improved by using radiometric rather than ICP-MS measurement of the ¹³⁷Cs isotope and by refining the Cs/Ba separation process. With these improvements, uncertainty in the age of a 60-year-old source decreases from 1.35 to 0.68 y.

Original language	English
Pages (from-to)	999-1019
Number of pages	21
Journal	Journal of Radioanalytical and Nuclear Chemistry
Volume	309
Issue number	3
DOIs	https://doi.org/10.1007/s10967-016-4712-x
State	Published - Sep 1 2016
Externally published	Yes

Keywords

Age dating
Cs ceramic
EDTA
Extraction chromatography
Nuclear forensics
RDD

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10.1007/s10967-016-4712-x

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title = "Age-dating methodology for 137Cs ceramic sources",

abstract = "Age-dating of 137Cs ceramic sources is shown to be a viable technology for nuclear forensics investigations. The 137Cs age-dating method in general, however, could be substantially improved by using radiometric rather than ICP-MS measurement of the 137Cs isotope and by refining the Cs/Ba separation process. With these improvements, uncertainty in the age of a 60-year-old source decreases from 1.35 to 0.68 y.",

keywords = "Age dating, Cs ceramic, EDTA, Extraction chromatography, Nuclear forensics, RDD",

author = "Steeb, \{Jennifer L.\} and Graczyk, \{Donald G.\} and Yifen Tsai and Mertz, \{Carol J.\} and Ashleigh Kimberlin and Chamberlain, \{David B.\}",

note = "Publisher Copyright: {\textcopyright} 2016, Akad{\'e}miai Kiad{\'o}, Budapest, Hungary.",

year = "2016",

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doi = "10.1007/s10967-016-4712-x",

language = "English",

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T1 - Age-dating methodology for 137Cs ceramic sources

AU - Steeb, Jennifer L.

AU - Graczyk, Donald G.

AU - Tsai, Yifen

AU - Mertz, Carol J.

AU - Kimberlin, Ashleigh

AU - Chamberlain, David B.

PY - 2016/9/1

Y1 - 2016/9/1

N2 - Age-dating of 137Cs ceramic sources is shown to be a viable technology for nuclear forensics investigations. The 137Cs age-dating method in general, however, could be substantially improved by using radiometric rather than ICP-MS measurement of the 137Cs isotope and by refining the Cs/Ba separation process. With these improvements, uncertainty in the age of a 60-year-old source decreases from 1.35 to 0.68 y.

AB - Age-dating of 137Cs ceramic sources is shown to be a viable technology for nuclear forensics investigations. The 137Cs age-dating method in general, however, could be substantially improved by using radiometric rather than ICP-MS measurement of the 137Cs isotope and by refining the Cs/Ba separation process. With these improvements, uncertainty in the age of a 60-year-old source decreases from 1.35 to 0.68 y.

KW - Age dating

KW - Cs ceramic

KW - EDTA

KW - Extraction chromatography

KW - Nuclear forensics

KW - RDD

UR - https://www.scopus.com/pages/publications/84955613997

U2 - 10.1007/s10967-016-4712-x

DO - 10.1007/s10967-016-4712-x

M3 - Article

AN - SCOPUS:84955613997

SN - 0236-5731

VL - 309

SP - 999

EP - 1019

JO - Journal of Radioanalytical and Nuclear Chemistry

JF - Journal of Radioanalytical and Nuclear Chemistry

IS - 3

ER -

Age-dating methodology for ¹³⁷Cs ceramic sources

Abstract

Keywords

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