Advancements in Amorphous Oxides For Electrocatalytic Carbon Dioxide Reduction

Electrocatalytic CO₂ reduction (ECR) is a crucial energy conversion technology that transforms CO₂ into value-added chemicals, reducing reliance on fossil fuels and advancing energy transitions. Designing high-performance catalysts is pivotal for widespread adoption of CO₂ reduction reactions, aiming for high activity, selectivity, and stability. Amorphous oxides represent a burgeoning frontier in this field, attracting attention due to their abundant active sites that refine the catalyst structure-performance relationship. This paper aims to provide an overview of recent advances in using amorphous oxides for ECR. We begin by introducing the basic theory of electrocatalytic CO₂ reduction, followed by discussing current synthesis approaches for amorphous oxides in CO₂ reduction, focusing on optimization strategies for these catalysts. Finally, we address challenges and future perspectives of amorphous oxides in ECR, aiming to foster the development of more efficient catalyst designs.