Additive manufacturing of liquid/gas diffusion layers for low-cost and high-efficiency hydrogen production

Jingke Mo, Ryan R. Dehoff, William H. Peter, Todd J. Toops, Johney B. Green, Feng Yuan Zhang

Research output: Contribution to journalArticlepeer-review

89 Scopus citations

Abstract

A low-cost additive manufacturing technology, electron beam melting (EBM), is employed for the first time to fabricate titanium liquid/gas diffusion media with high-corrosion resistances and well-controlled multifunctional parameters, including two-phase transport and high electric/thermal conductivities. Its application in proton exchange membrane electrolyzer cells (PEMECs) has been investigated in-situ with modular galvano (MG) and galvano electrochemical impedance spectroscopy (GEIS) and characterized ex-situ with SEM and XRD. Compared with conventional woven and sintered liquid/gas diffusion layers (LGDLs), much better performance is obtained with EBM-fabricated LGDLs due to a significant reduction of ohmic losses. The EBM technology components exhibited several distinct advantages in fabricating LGDLs: well-controllable pore morphology and structure, rapid prototyping, fast manufacturing, highly customizable design, and economic. In addition, by taking advantage of additive manufacturing, it is possible to fabricate complicated three-dimensional designs of virtually any shape from a digital model into one single solid object faster, cheaper, and easier, especially for titanium components. More importantly, this development will provide LGDLs with well-controllable pore morphologies, which will be valuable to develop sophisticated models of PEMECs with optimal and repeatable performance. Furthermore, it could lead to a manufacturing solution that greatly simplifies the PEMEC/fuel cell components.

Original languageEnglish
Pages (from-to)3128-3135
Number of pages8
JournalInternational Journal of Hydrogen Energy
Volume41
Issue number4
DOIs
StatePublished - Jan 30 2016

Funding

The authors greatly appreciate the support from U.S. Department of Energy''s National Energy Technology Laboratory under Award DE-FE0011585, and Office of Energy Efficiency and Renewable Energy, Advanced Manufacturing Office, under contract DE-AC05-00OR22725 with UT-Battelle, LLC. The authors also wish to express their appreciation to Stuart Steen, Dr. Bo Han, Zhengye, Kang, William Barnhill, Douglas Warnberg, and Rong Chen for their help.

Keywords

  • 3D printing
  • Electron beam melting additive manufacturing
  • Liquid/gas diffusion layers
  • Multifunctional materials
  • Proton exchange membrane electrolyzer cell

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