A rose bengal-functionalized porous organic polymer for carboxylative cyclization of propargyl alcohols with CO2

Xiaoxiao Yu; Zhenzhen Yang; Fengtao Zhang; Zhenghui Liu; Peng Yang; Hongye Zhang; Bo Yu; Yanfei Zhao; Zhimin Liu

doi:10.1039/c9cc07043e

A rose bengal-functionalized porous organic polymer for carboxylative cyclization of propargyl alcohols with CO₂

Xiaoxiao Yu, Zhenzhen Yang, Fengtao Zhang, Zhenghui Liu, Peng Yang, Hongye Zhang, Bo Yu, Yanfei Zhao, Zhimin Liu

Research output: Contribution to journal › Article › peer-review

47 Scopus citations

Abstract

A Rose bengal-functionalized porous organic polymer (RB-POP) was prepared with a specific surface area of up to 562 m² g^-1. In the presence of 1,8-diazabicyclo[5.4.0]undec-7-ene, RB-POP supported Ag(0) nanoparticles exhibited excellent performance for catalyzing cyclization of propargyl alcohols with CO₂ at 30 °C, achieving a TOF of 5000 h^-1, the highest value among the reported ones.

Original language	English
Pages (from-to)	12475-12478
Number of pages	4
Journal	Chemical Communications
Volume	55
Issue number	83
DOIs	https://doi.org/10.1039/c9cc07043e
State	Published - 2019
Externally published	Yes

Funding

We thank the National Key Research and Development Program of China (2018YFB0605801), the National Natural Science Foundation of China (No. 21673256), and the Chinese Academy of Sciences (QYZDY-SSW-SLH013-2), Beijing Municipal Science & Technology Commission (Z181100004218004) for the financial support.

Funders	Funder number
National Natural Science Foundation of China	21673256
Chinese Academy of Sciences	QYZDY-SSW-SLH013-2
Beijing Municipal Science and Technology Commission	Z181100004218004
National Basic Research Program of China (973 Program)	2018YFB0605801

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title = "A rose bengal-functionalized porous organic polymer for carboxylative cyclization of propargyl alcohols with CO2",

abstract = "A Rose bengal-functionalized porous organic polymer (RB-POP) was prepared with a specific surface area of up to 562 m2 g-1. In the presence of 1,8-diazabicyclo[5.4.0]undec-7-ene, RB-POP supported Ag(0) nanoparticles exhibited excellent performance for catalyzing cyclization of propargyl alcohols with CO2 at 30 °C, achieving a TOF of 5000 h-1, the highest value among the reported ones.",

author = "Xiaoxiao Yu and Zhenzhen Yang and Fengtao Zhang and Zhenghui Liu and Peng Yang and Hongye Zhang and Bo Yu and Yanfei Zhao and Zhimin Liu",

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year = "2019",

doi = "10.1039/c9cc07043e",

language = "English",

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T1 - A rose bengal-functionalized porous organic polymer for carboxylative cyclization of propargyl alcohols with CO2

AU - Yu, Xiaoxiao

AU - Yang, Zhenzhen

AU - Zhang, Fengtao

AU - Liu, Zhenghui

AU - Yang, Peng

AU - Zhang, Hongye

AU - Yu, Bo

AU - Zhao, Yanfei

AU - Liu, Zhimin

PY - 2019

Y1 - 2019

N2 - A Rose bengal-functionalized porous organic polymer (RB-POP) was prepared with a specific surface area of up to 562 m2 g-1. In the presence of 1,8-diazabicyclo[5.4.0]undec-7-ene, RB-POP supported Ag(0) nanoparticles exhibited excellent performance for catalyzing cyclization of propargyl alcohols with CO2 at 30 °C, achieving a TOF of 5000 h-1, the highest value among the reported ones.

AB - A Rose bengal-functionalized porous organic polymer (RB-POP) was prepared with a specific surface area of up to 562 m2 g-1. In the presence of 1,8-diazabicyclo[5.4.0]undec-7-ene, RB-POP supported Ag(0) nanoparticles exhibited excellent performance for catalyzing cyclization of propargyl alcohols with CO2 at 30 °C, achieving a TOF of 5000 h-1, the highest value among the reported ones.

UR - http://www.scopus.com/inward/record.url?scp=85073183833&partnerID=8YFLogxK

U2 - 10.1039/c9cc07043e

DO - 10.1039/c9cc07043e

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AN - SCOPUS:85073183833

SN - 1359-7345

VL - 55

SP - 12475

EP - 12478

JO - Chemical Communications

JF - Chemical Communications

IS - 83

ER -

A rose bengal-functionalized porous organic polymer for carboxylative cyclization of propargyl alcohols with CO₂

Abstract

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