A continuous-jet hydrate reactor for the formation of Co2 hydrate particles: Hydrate formation and dissolution in a high-pressure water tunnel facility

Costas Tsouris; David E. Riestenberg; Robert P. Warzinski; Ronald J. Lynn; Jorge F. Gabitto

A continuous-jet hydrate reactor for the formation of Co₂ hydrate particles: Hydrate formation and dissolution in a high-pressure water tunnel facility

Costas Tsouris, David E. Riestenberg, Robert P. Warzinski, Ronald J. Lynn, Jorge F. Gabitto

Chemical Process Scale Up

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review

Abstract

A three-phase continuous-jet hydrate reactor (CJHR) is developed to produce dense CO₂ hydrate particles for the purpose of ocean CO₂ sequestration. The CJHR injector/reactor is described and experimental results using a High-pressure Water Tunnel Facility at the National Energy Technology Laboratory are be presented. The inputs to the reactor are liquid CO₂ and seawater and the output is composite particles containing CO₂ hydrate, unreacted liquid CO₂, and seawater. Injections of composite particles are performed at pressures equivalent to 1200-1800 m depth and temperatures of 3°-5°C. CO₂ hydrate dissolution at intermediate ocean depths is modeled using pseudohomogeneous and heterogeneous mass-transfer models to predict dissolution rates under different operating conditions. This is an abstract of a paper presented at the AIChE Annual Meeting and Fall Showcase (Cincinnati, OH 10/30/2005-11/4/2005).

Original language	English
Title of host publication	05AIChE
Subtitle of host publication	2005 AIChE Annual Meeting and Fall Showcase, Conference Proceedings
Publisher	American Institute of Chemical Engineers
ISBN (Print)	0816909962, 9780816909964
State	Published - 2005
Event	05AIChE: 2005 AIChE Annual Meeting and Fall Showcase - Cincinnati, OH, United States Duration: Oct 30 2005 → Nov 4 2005

Publication series

Name	AIChE Annual Meeting Conference Proceedings
Volume	2005

Conference

Conference	05AIChE: 2005 AIChE Annual Meeting and Fall Showcase
Country/Territory	United States
City	Cincinnati, OH
Period	10/30/05 → 11/4/05

Cite this

Tsouris, C., Riestenberg, D. E., Warzinski, R. P., Lynn, R. J., & Gabitto, J. F. (2005). A continuous-jet hydrate reactor for the formation of Co₂ hydrate particles: Hydrate formation and dissolution in a high-pressure water tunnel facility. In 05AIChE: 2005 AIChE Annual Meeting and Fall Showcase, Conference Proceedings (AIChE Annual Meeting Conference Proceedings; Vol. 2005). American Institute of Chemical Engineers.

Tsouris, Costas ; Riestenberg, David E. ; Warzinski, Robert P. et al. / A continuous-jet hydrate reactor for the formation of Co₂ hydrate particles : Hydrate formation and dissolution in a high-pressure water tunnel facility. 05AIChE: 2005 AIChE Annual Meeting and Fall Showcase, Conference Proceedings. American Institute of Chemical Engineers, 2005. (AIChE Annual Meeting Conference Proceedings).

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title = "A continuous-jet hydrate reactor for the formation of Co2 hydrate particles: Hydrate formation and dissolution in a high-pressure water tunnel facility",

abstract = "A three-phase continuous-jet hydrate reactor (CJHR) is developed to produce dense CO2 hydrate particles for the purpose of ocean CO2 sequestration. The CJHR injector/reactor is described and experimental results using a High-pressure Water Tunnel Facility at the National Energy Technology Laboratory are be presented. The inputs to the reactor are liquid CO2 and seawater and the output is composite particles containing CO2 hydrate, unreacted liquid CO2, and seawater. Injections of composite particles are performed at pressures equivalent to 1200-1800 m depth and temperatures of 3°-5°C. CO2 hydrate dissolution at intermediate ocean depths is modeled using pseudohomogeneous and heterogeneous mass-transfer models to predict dissolution rates under different operating conditions. This is an abstract of a paper presented at the AIChE Annual Meeting and Fall Showcase (Cincinnati, OH 10/30/2005-11/4/2005).",

author = "Costas Tsouris and Riestenberg, {David E.} and Warzinski, {Robert P.} and Lynn, {Ronald J.} and Gabitto, {Jorge F.}",

year = "2005",

language = "English",

isbn = "0816909962",

series = "AIChE Annual Meeting Conference Proceedings",

publisher = "American Institute of Chemical Engineers",

booktitle = "05AIChE",

note = "05AIChE: 2005 AIChE Annual Meeting and Fall Showcase ; Conference date: 30-10-2005 Through 04-11-2005",

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Tsouris, C, Riestenberg, DE, Warzinski, RP, Lynn, RJ & Gabitto, JF 2005, A continuous-jet hydrate reactor for the formation of Co₂ hydrate particles: Hydrate formation and dissolution in a high-pressure water tunnel facility. in 05AIChE: 2005 AIChE Annual Meeting and Fall Showcase, Conference Proceedings. AIChE Annual Meeting Conference Proceedings, vol. 2005, American Institute of Chemical Engineers, 05AIChE: 2005 AIChE Annual Meeting and Fall Showcase, Cincinnati, OH, United States, 10/30/05.

A continuous-jet hydrate reactor for the formation of Co₂ hydrate particles: Hydrate formation and dissolution in a high-pressure water tunnel facility. / Tsouris, Costas; Riestenberg, David E.; Warzinski, Robert P. et al.
05AIChE: 2005 AIChE Annual Meeting and Fall Showcase, Conference Proceedings. American Institute of Chemical Engineers, 2005. (AIChE Annual Meeting Conference Proceedings; Vol. 2005).

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review

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AB - A three-phase continuous-jet hydrate reactor (CJHR) is developed to produce dense CO2 hydrate particles for the purpose of ocean CO2 sequestration. The CJHR injector/reactor is described and experimental results using a High-pressure Water Tunnel Facility at the National Energy Technology Laboratory are be presented. The inputs to the reactor are liquid CO2 and seawater and the output is composite particles containing CO2 hydrate, unreacted liquid CO2, and seawater. Injections of composite particles are performed at pressures equivalent to 1200-1800 m depth and temperatures of 3°-5°C. CO2 hydrate dissolution at intermediate ocean depths is modeled using pseudohomogeneous and heterogeneous mass-transfer models to predict dissolution rates under different operating conditions. This is an abstract of a paper presented at the AIChE Annual Meeting and Fall Showcase (Cincinnati, OH 10/30/2005-11/4/2005).

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BT - 05AIChE

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Tsouris C, Riestenberg DE, Warzinski RP, Lynn RJ, Gabitto JF. A continuous-jet hydrate reactor for the formation of Co₂ hydrate particles: Hydrate formation and dissolution in a high-pressure water tunnel facility. In 05AIChE: 2005 AIChE Annual Meeting and Fall Showcase, Conference Proceedings. American Institute of Chemical Engineers. 2005. (AIChE Annual Meeting Conference Proceedings).

A continuous-jet hydrate reactor for the formation of Co₂ hydrate particles: Hydrate formation and dissolution in a high-pressure water tunnel facility

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