A computational meta-analysis of UCl3 cyclic voltammograms in LiCl-KCl electrolyte

Riley M. Cumberland; Man Sung Yim

doi:10.1149/2.033404jes

A computational meta-analysis of UCl₃ cyclic voltammograms in LiCl-KCl electrolyte

Riley M. Cumberland, Man Sung Yim

Research output: Contribution to journal › Article › peer-review

18 Scopus citations

Abstract

As a way to characterize the values of key parameters for modeling electrochemical transport of elements in a molten salt system, a meta-analysis of CV reduction peaks for UCl₃ in LiCl-KCl eutectic was performed. Published CV data was fit using least squares fitting software coupled with electrochemical simulation software. The analysis yielded estimates of apparent standard potential, the diffusion coefficient, and the exchange current density for each reaction. The results for the UCl₃ reduction peak matched well with existing data.

Original language	English
Pages (from-to)	D147-D149
Journal	Journal of the Electrochemical Society
Volume	161
Issue number	4
DOIs	https://doi.org/10.1149/2.033404jes
State	Published - 2014
Externally published	Yes

Funding

This work was supported by Korea Research Foundation under the contact number 2011-0031839. The authors would also like to acknowledge the support from Prof. Il Soon Hwang of Seoul National University who provided the REFIN code.

Funders	Funder number
Korea Research Foundation	2011-0031839
Seoul National University
Korean Foundation for Cancer Research

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abstract = "As a way to characterize the values of key parameters for modeling electrochemical transport of elements in a molten salt system, a meta-analysis of CV reduction peaks for UCl3 in LiCl-KCl eutectic was performed. Published CV data was fit using least squares fitting software coupled with electrochemical simulation software. The analysis yielded estimates of apparent standard potential, the diffusion coefficient, and the exchange current density for each reaction. The results for the UCl3 reduction peak matched well with existing data.",

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AB - As a way to characterize the values of key parameters for modeling electrochemical transport of elements in a molten salt system, a meta-analysis of CV reduction peaks for UCl3 in LiCl-KCl eutectic was performed. Published CV data was fit using least squares fitting software coupled with electrochemical simulation software. The analysis yielded estimates of apparent standard potential, the diffusion coefficient, and the exchange current density for each reaction. The results for the UCl3 reduction peak matched well with existing data.

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A computational meta-analysis of UCl₃ cyclic voltammograms in LiCl-KCl electrolyte

Abstract

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