A compact furnace to support in situ neutron imaging of hydrogen dynamics in yttrium hydride moderators

James Torres, Alexander Long, D. Travis Carver, Christopher Matthews, Sven Vogel, Tyler Smith, Caitlin Kohnert, Erik Luther, Holly Trellue, Aditya Shivprasad

Research output: Contribution to journalArticlepeer-review

Abstract

A compact, nuclear microreactor that utilizes low-enriched uranium fuel is a promising solution to meet U.S. energy demands in nonconventional nuclear markets such as remote and decentralized energy grids. Yttrium hydride (YHx) is a potential moderator material for a microreactor design that reduces the amount of required fuel and provides superior retention of hydrogen at high reactor operating temperatures. Hydrogen diffusion properties in YHx are highly sought after for computer model validation and reactor prototyping. To characterize hydrogen diffusion, a compact dual-zone furnace was developed at Los Alamos National Laboratory and analyzed via neutron imaging at the Los Alamos Neutron Science Center (LANSCE). The goal of these measurements is to assess hydrogen diffusion in YHx samples as a function of applied temperature gradients. Included herein is recent progress in technique and furnace developments as well as initial results from concentration- and temperature-gradient measurements at LANSCE. Graphical abstract: Compact dual-zone furnace at LANSCE (Figure presented.)

Original languageEnglish
Pages (from-to)1227-1233
Number of pages7
JournalMRS Advances
Volume9
Issue number16
DOIs
StatePublished - Aug 2024

Funding

This work was supported by the U.S. Department of Energy Microreactor Program and authored by Battelle Energy Alliance, LLC, under Contract No. DE-AC07-05-ID14517 with the U.S. Department of Energy, Office of Nuclear Energy. Los Alamos National Laboratory, an affirmative action/equal opportunity employer, is operated by Triad National Security LLC, for the National Nuclear Security Administration of the U.S. Department of Energy under Contract No. 89233218CNA000001. A portion of this research used resources at the High Flux Isotope Reactor, a DOE Office of Science User Facility operated by the Oak Ridge National Laboratory. The authors thank Bekki Mills for helpful feedback. This work was supported by the U.S. Department of Energy Microreactor Program and authored by Battelle Energy Alliance, LLC, under Contract No. DE-AC07-05-ID14517 with the U.S. Department of Energy, Office of Nuclear Energy. A portion of this research used resources at the High Flux Isotope Reactor, a DOE Office of Science User Facility operated by the Oak Ridge National Laboratory.

FundersFunder number
Oak Ridge National Laboratory
Los Alamos National Laboratory
Office of Science
Office of Nuclear Energy
U.S. Department of EnergyDE-AC07-05-ID14517
U.S. Department of Energy
National Nuclear Security Administration89233218CNA000001
National Nuclear Security Administration

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