Isotope Sci & Eng Directorate

2025

Validation of a general-use high flux isotope reactor–specific metaheuristic optimization framework for isotope production target design

Salyer, C., Bogetic, S. & Griswold, J., Feb 2025, In: Applied Radiation and Isotopes. 216, 111592.

Research output: Contribution to journal › Article › peer-review

2024

Absolute Branching Ratios of Prominent γ Rays Following α Decay of ²³³U

Gray, T. J., Allmond, J. M., Evans, L. G., Roach, B. D., King, T. T. & Rasco, B. C., Feb 2024, In: Nuclear Data Sheets. 193, p. 88-94 7 p.

Research output: Contribution to journal › Article › peer-review

Advancing Elemental and Isotopic Analysis of Uranium Mineral Inclusions: Rapid Screening via Laser-Induced Breakdown Spectroscopy and High-Resolution Laser Ablation-ICP-MS Mapping

Andrews, H. B., Derrick Quarles, C., Bradley, V. C., Spano, T. L., Petrus, J. A., Paul, B., Alex Zirakparvar, N., Dunlap, D. R., Hexel, C. R. & Manard, B. T., Jan 2024, In: Microchemical Journal. 196, 109605.

Research output: Contribution to journal › Article › peer-review

5 Scopus citations

Analytical capabilities for iodine detection: Review of possibilities for different applications

Riley, B. J., Beck, C. L., Evarts, J. S., Chong, S., Lines, A. M., Felmy, H. M., McFarlane, J., Andrews, H. B., Bryan, S. A., McHugh, K. C., Cunningham, H. S., Asmussen, R. M., Dhas, J. A., Zhu, Z., Crum, J. V., Shen, S. D., McCloy, J. S. & Heiden, Z. M., Aug 1 2024, In: AIP Advances. 14, 8, 080701.

Research output: Contribution to journal › Review article › peer-review

1 Scopus citations

Automated Calibration for Rapid Optical Spectroscopy Sensor Development for Online Monitoring

Andrews, H. B. & Sadergaski, L. R., Nov 22 2024, In: ACS Sensors. 9, 11, p. 6257-6264 8 p.

Research output: Contribution to journal › Article › peer-review

Open Access

Changing absorption intensity ratios for methylene violet Bernthsen in normal alcohols and at different temperatures

Villamizar-Mendoza, S., Reel, J., Kimberlin, A., Taylor, J., Howe, M., Rowe, G. & Fetterolf, M., Apr 16 2024, In: Chemical Physics Letters. 841, 141167.

Research output: Contribution to journal › Article › peer-review

Characterization of fluidized bed chemical vapor deposition ZrC coatings on PyC/YSZ kernels deposited under differing conditions

Doyle, P., Lopez-Honorato, E., Vasudevamurthy, G., Miller, J., Meyer, H. & Gerczak, T., Jun 2024, In: Journal of Nuclear Materials. 594, 155019.

Research output: Contribution to journal › Article › peer-review

Collector probe analysis of tungsten transport to the far-SOL from the DIII-D SAS-VW divertor experiment

Messer, S. H., Mateja, J. D., Nichols, J. H., Cacheris, A., Duran, J. D., Zamperini, S. A., Sinclair, G., Donovan, D., Abrams, T., Odstrcil, T., Ren, J., Garcia, W., Unterberg, E. A., Stangeby, P. C., Rudakov, D. L., Elder, J. D. & Watkins, J., Mar 2024, In: Nuclear Materials and Energy. 38, 101566.

Research output: Contribution to journal › Article › peer-review

Open Access

2 Scopus citations

Comparing Sensor Fusion and Multimodal Chemometric Models for Monitoring U(VI) in Complex Environments Representative of Irradiated Nuclear Fuel

Sadergaski, L. R., Andrews, H. B. & Wilson, B. A., Jan 30 2024, In: Analytical Chemistry. 96, 4, p. 1759-1766 8 p.

Research output: Contribution to journal › Article › peer-review

3 Scopus citations

Conducting MUSiC Modeling Studies

Marshall, W. J., Brandt, M. T., Mulig, L. M., Greene, T. M., Blair, S. R. & Shaw, A. M., 2024, In: Transactions of the American Nuclear Society. 130, 1, p. 806-809 4 p.

Research output: Contribution to journal › Conference article › peer-review

Current Overview of Neutron Moderator Thermal Scattering Kernels for HALEU-Fueled Advanced Reactors

Al-Qasir, I. I., Reed, K. L., Marshall, W. J., Dupont, M. N., Chapman, C. W., Hartanto, D., Metwally, W. A. & Wieselquist, W. A., 2024, In: Transactions of the American Nuclear Society. 130, 1, p. 750-753 4 p.

Research output: Contribution to journal › Conference article › peer-review

Decay studies of the β-delayed neutron emitters Br 87 and Br 88 measured by means of the Modular Total Absorption Spectrometer at ORNL HRIBF

Stepaniuk, M., Karny, M., Fijałkowska, A., Rykaczewski, K. P., Rasco, B. C., Grzywacz, R. K., Wolińska-Cichocka, M., Allmond, J. M., Batchelder, J. C., Bingham, C., Blackmon, J. C., Brewer, N. T., Go, S., Goetz, K. C., Gross, C. J., Johnson, J., Jost, C. U., Hamilton, J. H., King, T. T. & Kolos, K. & 15 others, Matta, J. T., Miernik, K., Madurga, M., Miller, D., Nesaraja, C. D., Padgett, S., Paulauskas, S. V., Rajabali, M. M., Stracener, D. W., Spejewski, E. H., Taylor, S., Wang, E. H., Winger, J. A., Xiao, Y. & Zganjar, E. F., Nov 2024, In: Physical Review C. 110, 5, 054321.

Research output: Contribution to journal › Article › peer-review

Density Measurements of Molten LiF-BeF₂ and LiF-BeF₂-LaF₃ Salt Mixtures by Neutron Radiography

Moon, J., McFarlane, J., Andrews, H. B., Robb, K. R., Ross, M., Sulejmanovic, D., Zhang, Y., Stringfellow, E., Agca, C., Schorne-Pinto, J. & Besmann, T. M., 2024, (Accepted/In press) In: ACS Omega.

Research output: Contribution to journal › Article › peer-review

Open Access

Development of ²²⁵Ac-doped biocompatible nanoparticles for targeted alpha therapy

Toro-González, M., Akingbesote, N., Bible, A., Pal, D., Sanders, B., Ivanov, A. S., Jansone-Popova, S., Popovs, I., Benny, P., Perry, R. & Davern, S., Dec 2024, In: Journal of nanobiotechnology. 22, 1, 306.

Research output: Contribution to journal › Article › peer-review

Open Access

Disrupting the Hofmeister bias in salt liquid-liquid extraction with an arylethynyl bisurea anion receptor

Fargher, H. A., Delmau, L. H., Bryantsev, V. S., Haley, M. M., Johnson, D. W. & Moyer, B. A., Mar 7 2024, In: Chemical Science. 15, 14, p. 5311-5318 8 p.

Research output: Contribution to journal › Article › peer-review

Open Access

DYNAMIC RESPONSE OF A PIVOT-MOUNTED SQUEEZE FILM DAMPER: MEASUREMENTS AND PREDICTIONS

Kasprzyk, M. & Delgado, A., 2024, Structures and Dynamics - Aerodynamics Excitation and Damping; Bearing and Seal Dynamics; Emerging Methods in Engineering Design, Analysis, and Additive Manufacturing. American Society of Mechanical Engineers (ASME), V10AT22A003. (Proceedings of the ASME Turbo Expo; vol. 10A).

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review

Effect of Decay Time on Criticality Safety Analyses for High-Burnup and Extended Enrichment Fuels

Shaw, A. M., Metwally, W. A., Dupont, M. N., Marshall, W. J., Celik, C., Karriem, V., Lang, A. & Fassino, K. L., 2024, In: Transactions of the American Nuclear Society. 130, 1, p. 794-797 4 p.

Research output: Contribution to journal › Conference article › peer-review

Effect of f-element complexation on the radiolysis of 2-ethylhexylphosphonic acid mono-2-ethylhexyl ester (HEH[EHP])

Mezyk, S. P., Baxter, M., Celis-Barros, C., Grimes, T. S., Zalupski, P. R., Rae, C., Zarzana, C. A., Cook, A. R. & Horne, G. P., Feb 26 2024, In: Dalton Transactions. 53, 16, p. 6881-6891 11 p.

Research output: Contribution to journal › Article › peer-review

Electrochemically Assisted Single Crystal Growth of Reduced Preyssler Polyoxometalates Decorated with M²⁺ (M = Co, Ni) and Cubane-Like Ni₄O₄ Units

Sheriff, K., Sulejmanovic, D., Jun, J., Cannon, W., Petta, L., Phillips, J., McMillen, C. & Hwu, S., Sep 23 2024, In: Inorganic Chemistry. 63, 38, p. 17584-17597 14 p.

Research output: Contribution to journal › Article › peer-review

Evaluating Optical Techniques to Characterize Solid State Samples for the Pu-238 Supply Program

Sadergaski, L., Andrews, H., Sharpe, J., Parkison, A. & Myhre, K., Jan 2024

Research output: Other contribution › Technical Report

Evaluation of Corrosion Behavior of Various Fe- and Ni-Based Alloys in Molten Li₂BeF₄ (FLiBe)

Sankar, K. M., Keiser, J. R., Sulejmanovic, D., Lowe, T. M. & Singh, P. M., 2024, In: Nuclear Technology. 210, 3, p. 391-408 18 p.

Research output: Contribution to journal › Article › peer-review

Fungal elemental profiling unleashed through rapid laser-induced breakdown spectroscopy (LIBS)

Rush, T. A., Wymore, A. M., Rodríguez, M., Jawdy, S., Vilgalys, R. J., Martin, M. Z. & Andrews, H. B., Sep 2024, In: mSystems. 9, 9

Research output: Contribution to journal › Article › peer-review

Open Access

Generic and facile mechanochemical access to versatile lattice-confined Pd(ii)-based heterometallic sites

Tegudeer, Z., Moon, J., Wright, J., Das, M., Rubasinghege, G., Xu, W. & Gao, W. Y., 2024, (Accepted/In press) In: Chemical Science.

Research output: Contribution to journal › Article › peer-review

Open Access

Harnessing the Unique Properties of Berkelium in its Separation from other f-Elements and Fission Products

Du, M. & Thakur, P., 2024, In: Transactions of the American Nuclear Society. 130, 1, p. 388-391 4 p.

Research output: Contribution to journal › Conference article › peer-review

How irradiation promotes intergranular stress corrosion crack initiation

Was, G. S., Bahn, C. B., Busby, J., Cui, B., Farkas, D., Gussev, M., Rigen He, M., Hesterberg, J., Jiao, Z., Johnson, D., Kuang, W., McMurtrey, M., Robertson, I., Sinjlawi, A., Song, M., Stephenson, K., Sun, K., Swaminathan, S., Wang, M. & West, E., Jun 2024, In: Progress in Materials Science. 143, 101255.

Research output: Contribution to journal › Review article › peer-review

Open Access

7 Scopus citations

Improving understanding of NpO₂ and Np₂O₅ through vibrational spectroscopy

Gilson, S. E., Sadergaski, L. R. & Parkison, A. J., Nov 2024, In: Journal of Solid State Chemistry. 339, 124954.

Research output: Contribution to journal › Article › peer-review

Insights into Tetravalent Np Speciation in HNO₃ through Spectroelectrochemistry and Multivariate Analysis

Gilson, S. E., Andrews, H. B., Sadergaski, L. R. & Parkison, A. J., Oct 29 2024, In: ACS Omega. 9, 43, p. 43547-43556 10 p.

Research output: Contribution to journal › Article › peer-review

Open Access

Investigating a Potential Hafnium Bias in SCALE

Greene, T. M., Marshall, W. J., Brandt, M. T., Mulig, L. M., Blair, S. R. & Shaw, A. M., 2024, In: Transactions of the American Nuclear Society. 130, 1, p. 822-825 4 p.

Research output: Contribution to journal › Conference article › peer-review

Laser Ablation Plasmas and Spectroscopy for Nuclear Applications

Kwapis, E. H., Borrero, J., Latty, K. S., Andrews, H. B., Phongikaroon, S. “. & Hartig, K. C., Jan 2024, In: Applied Spectroscopy. 78, 1, p. 9-55 47 p.

Research output: Contribution to journal › Review article › peer-review

16 Scopus citations

Leveraging Calibration Transfer Techniques for Remote Monitoring of Samarium and Europium in LiCl Using Laser-Induced Florescence Spectroscopy for Radioisotope Production Applications

Andrews, H. B., Moon, J. & Sadergaski, L. R., 2024, (Accepted/In press) In: Industrial and Engineering Chemistry Research.

Research output: Contribution to journal › Article › peer-review

1 Scopus citations

Mapping of uranium particles on J-type swipes with microextraction-ICP-MS

Bradley, V. C., Burleson, J., Andrews, H. B., Thompson, C. V., Spano, T. L., Dunlap, D. R., Zirakparvar, N. A., Ticknor, B. W., Hexel, C. R. & Manard, B. T., Feb 20 2024, In: Analyst. 149, 8, p. 2244-2251 8 p.

Research output: Contribution to journal › Article › peer-review

Open Access

1 Scopus citations

MIP-4 is Induced by Bleomycin and Stimulates Cell Migration Partially via Nir-1 Receptor

Pacurari, M., Cox, I., Bible, A. N. & Davern, S., 2024, In: Biochemistry Research International. 2024, 5527895.

Research output: Contribution to journal › Article › peer-review

Open Access

Modeling turbulent impurity transport in the SOL of DIII-D with a reduced model

Zamperini, S., Nichols, J. H., Odstrcil, T., Abrams, T., Boedo, J. A., Elder, J. D., Rudakov, D. L., Donovan, D. C., Duran, J. D. & Huang, A., May 2024, In: Plasma Physics and Controlled Fusion. 66, 5, 055003.

Research output: Contribution to journal › Article › peer-review

2 Scopus citations

Observation of a promethium complex in solution

Driscoll, D. M., White, F. D., Pramanik, S., Einkauf, J. D., Ravel, B., Bykov, D., Roy, S., Mayes, R. T., Delmau, L. H., Cary, S. K., Dyke, T., Miller, A., Silveira, M., VanCleve, S. M., Davern, S. M., Jansone-Popova, S., Popovs, I. & Ivanov, A. S., May 23 2024, In: Nature. 629, 8013, p. 819-823 5 p.

Research output: Contribution to journal › Article › peer-review

Open Access

8 Scopus citations

On Estimating Uncertainty in Integral Benchmarks due to Inconsistencies in Geometrical Measurements

Worrell, K., Sobes, V. & Marshall, W., 2024, In: Transactions of the American Nuclear Society. 130, 1, p. 742-744 3 p.

Research output: Contribution to journal › Conference article › peer-review

Post-irradiation examination of commercial tantalum alloys following neutron irradiation

Massey, C. P., Goetz, C. K., Lin, Y. R., Werden, J., Curlin, S., Siggillino, T. I., Zinkle, S. J. & Busby, J. T., Apr 1 2024, In: Journal of Nuclear Materials. 591, 154906.

Research output: Contribution to journal › Article › peer-review

1 Scopus citations

Precision Atomistic Structures of Actinium-/Radium-/Barium-Doped Lanthanide Nanoconstructs for Radiotherapeutic Applications

Goswami, M., Toro-González, M., Moon, J. & Davern, S., 2024, (Accepted/In press) In: ACS Nano.

Research output: Contribution to journal › Article › peer-review

Open Access

Probing the interface structure of block copolymer compatibilizers in semicrystalline polymer blends

Tang, X., Liu, C., Chen, J., Kumar, R., Bowland, C. C., Saito, T., Dial, B. E., Keum, J. K., Do, C. & Chen, X. C., Apr 10 2024, In: Journal of Applied Polymer Science. 141, 14, e55178.

Research output: Contribution to journal › Article › peer-review

Open Access

2 Scopus citations

Proceedings for the Workshop on Applied Nuclear Data Activities 2024

Gott, M., Humrickhouse, P., Loughlin, M., Mertyurek, U. & Brown, J., Jul 2024

Research output: Other contribution › Technical Report

PYTA: a universal chelator for advancing the theranostic palette of nuclear medicine

Simms, M. E., Li, Z., Sibley, M. M., Ivanov, A. S., Lara, C. M., Johnstone, T. C., Kertesz, V., Fears, A., White, F. D., Thorek, D. L. J. & Thiele, N. A., Jun 17 2024, In: Chemical Science. 15, 29, p. 11279-11286 8 p.

Research output: Contribution to journal › Article › peer-review

Open Access

2 Scopus citations

Quantifying platinum binding on protein-functionalized magnetic microparticles using single particle-ICP-TOF-MS

Bradley, V. C., Manard, B. T., Hendriks, L., Dunlap, D. R., Bible, A. N., Sedova, A., Saint-Vincent, P., Sanders, B. C. & Andrews, H. B., 2024, (Accepted/In press) In: Analytical Methods.

Research output: Contribution to journal › Article › peer-review

Open Access

Rapid in situ nutrient element distribution in plants and soils using laser-induced breakdown spectroscopy (LIBS)

Andrews, H. B., Martin, M. Z., Wymore, A. M. & Kalluri, U. C., Feb 2024, In: Plant and Soil. 495, 1-2, p. 3-12 10 p.

Research output: Contribution to journal › Article › peer-review

Open Access

5 Scopus citations

Remote Sensing of Nitric Acid and Temperature via Design of Experiments, Chemometrics, and Raman Spectroscopy

Russell, D. V., Sadergaski, L. R., Einkauf, J. D., Delmau, L. H. & Burns, J. D., Nov 12 2024, In: ACS Omega. 9, 45, p. 45600-45609 10 p.

Research output: Contribution to journal › Article › peer-review

Open Access

Review of Available Critical Experiments and Critical Experiments Facilities to Perform High-Assay Low-Enriched Uranium Fuel Transport Validation for Advanced Reactor Deployment

Dupont, M. N., Fassino, K. L. R., Marshall, W. J., Metwally, W. A. & Wieselquist, W. A., 2024, In: Transactions of the American Nuclear Society. 130, 1, p. 784-787 4 p.

Research output: Contribution to journal › Conference article › peer-review

Shape-Selective Supramolecular Capsules for Actinide Precipitation and Separation

O’Connell-Danes, J., Ngwenya, B. T., Morrison, C. A., Nichol, G. S., Delmau, L. H. & Love, J. B., Feb 26 2024, In: JACS Au. 4, 2, p. 798-806 9 p.

Research output: Contribution to journal › Article › peer-review

Open Access

4 Scopus citations

Simultaneous Separation of Protactinium-230 and Uranium-230 Isotopes from a Proton-Irradiated Thorium Matrix

Du, M., Dyer, T. & Thakur, P., Apr 16 2024, In: Analytical Chemistry. 96, 15, p. 5906-5912 7 p.

Research output: Contribution to journal › Article › peer-review

Smooth trends in fermium charge radii and the impact of shell effects

Warbinek, J., Rickert, E., Raeder, S., Albrecht-Schönzart, T., Andelic, B., Auler, J., Bally, B., Bender, M., Berndt, S., Block, M., Brizard, A., Chauveau, P., Cheal, B., Chhetri, P., Claessens, A., de Roubin, A., Devlin, C., Dorrer, H., Düllmann, C. E. & Ezold, J. & 55 others, Ferrer, R., Gadelshin, V., Gaiser, A., Giacoppo, F., Goriely, S., Gutiérrez, M. J., Harvey, A., Hasse, R., Heinke, R., Heßberger, F. P., Hilaire, S., Kaja, M., Kaleja, O., Kieck, T., Kim, E. K., Kneip, N., Köster, U., Kraemer, S., Laatiaoui, M., Lantis, J., Lecesne, N., Loria Basto, A. T., Mistry, A. K., Mokry, C., Moore, I., Murböck, T., Münzberg, D., Nazarewicz, W., Niemeyer, T., Nothhelfer, S., Péru, S., Raggio, A., Reinhard, P. G., Renisch, D., Rey-Herme, E., Romans, J., Romero Romero, E., Runke, J., Ryssens, W., Savajols, H., Schneider, F., Sperling, J., Stemmler, M., Studer, D., Thörle-Pospiech, P., Trautmann, N., Urquiza-González, M., van Beek, K., Van Cleve, S., Van Duppen, P., Vandebrouck, M., Verstraelen, E., Walther, T., Weber, F. & Wendt, K., Oct 1 2024, In: Nature. 634, 8036, p. 1075-1079 5 p.

Research output: Contribution to journal › Article › peer-review

Open Access

Spatially Resolved Raman Spectroscopic Investigation of Uranyl Fluoride: A Case Study in the Importance of Instrument Optimization

Spano, T. L., Andrews, H. B., Miskowiec, A., Beiswenger, T. N. & Manard, B. T., 2024, (Accepted/In press) In: Applied Spectroscopy.

Research output: Contribution to journal › Article › peer-review

Structure and bonding of a radium coordination compound in the solid state

White, F. D., Thiele, N. A., Simms, M. E. & Cary, S. K., Feb 2024, In: Nature Chemistry. 16, 2, p. 168-172 5 p.

Research output: Contribution to journal › Article › peer-review

Open Access

2 Scopus citations

Thermochemical Non-Equilibrium Modeling in a Continuous-Galerkin, Finite-Element Framework

Nutter, N. F., Sanjaya, D. P., Glasby, R., Stefanski, D., Erwin, T. & Curtis, F., 2024, AIAA Aviation Forum and ASCEND, 2024. American Institute of Aeronautics and Astronautics Inc, AIAA, (AIAA Aviation Forum and ASCEND, 2024).

Research output: Chapter in Book/Report/Conference proceeding › Conference contribution › peer-review

Isotope Sci & Eng Directorate

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